RT Journal Article T1 Core and End-Capped Engineering as a Powerful Tool in the Search of Long-Term High-Performance Dye-Sensitized Solar Cells A1 Alonso Navarro, Matías J. A1 Franco, Santiago A1 Suárez Blas, Fátima A1 Andreu, Raquel A1 Orduna, Jesús A1 Ramos, M. Mar A1 Segura Castedo, José Luis AB In the search of new electroactive organic dyes in dye-sensitized solar cells technology, a series of D-π-A assemblies, named as TA-BTD-CNCOOH, OMeTA-BTD-CNCOOH, TA-Y6-CNCOOH, and OMeTA-Y6-CNCOOH is rationally designed and synthesized, in which precise modifications have been carried out in order to obtain structure-performance relations in the field of dye-sensitized solar cells. After careful evaluation of the photophysical and electrochemical properties of these semiconductors, these systems are applied as active materials, showing high performance with power conversion efficiency maximum values of 9.05% and 18.5% for outdoor and indoor conditions, respectively. In addition, the best material of these organic architectures, TA-BTD-CNCOOH, shows an excellent long-term stability, up to 3,360 h, with no significant variance in its performance over time. PB Wiley-VCH YR 2025 FD 2025-09-05 LK https://hdl.handle.net/20.500.14352/124391 UL https://hdl.handle.net/20.500.14352/124391 LA eng NO Alonso‐Navarro, Matías J., et al. «Core and End‐Capped Engineering as a Powerful Tool in the Search of Long‐Term High‐Performance Dye‐Sensitized Solar Cells». ChemSusChem, septiembre de 2025, p. e202501564. DOI.org (Crossref), https://doi.org/10.1002/cssc.202501564. NO MICINN NO Comunidad de Madrid DS Docta Complutense RD 17 dic 2025