RT Journal Article
T1 Linear optical properties of one-dimensional Frenkel exciton systems with intersite energy correlations
A1 Malyshev, Andrey
A1 Rodriguez, A.
A1 Domínguez-Adame Acosta, Francisco
AB We analyze the effects of intersite energy correlations on the linear optical properties of one-dimensional disordered Frenkel exciton systems. The absorption linewidth and the factor of radiative rate enhancement are studied as a function of the correlation length of the disorder. Thr absorption line width monotonously approaches the seeding degree of disorder on increasing the correlation length. On the contrary, the factor of radiative rate enhancement shows a nonmonotonous trend, indicating a complicated scenario of the exciton localization in correlated systems. The concept of coherently bound molecules is exploited to explain the numerical results, showing good agreement with theory. Some recent experiments are discussed in the light of the present theory. [S0163-1829(99)07343-9].
PB American Physical Society
SN 1098-0121
YR 1999
FD 1999-11-15
LK https://hdl.handle.net/20.500.14352/59358
UL https://hdl.handle.net/20.500.14352/59358
LA eng
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NO © 1999 The American Physical Society.This work was supported by CAM under Project No. 07N/0034/1998. V. A. M. thanks UCM for support under project ‘‘ Sabáticos Complutense.’’
NO CAM
NO UCM-Sabáticos Complutenses
DS Docta Complutense
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