RT Journal Article T1 Graphene-Based Microbots for Toxic Heavy Metal Removal and Recovery from Water A1 Vilela García, Diana A1 Parmar, Jemish A1 Zeng, Yongfei A1 Zhao, Yanli A1 Sánchez, Samuel AB Heavy metal contamination in water is a serious risk to the public health and other life forms on earth. Current research in nanotechnology is developing new nanosystems and nanomaterials for the fast and efficient removal of pollutants and heavy metals from water. Here, we report graphene oxide-based microbots (GOx-microbots) as active self-propelled systems for the capture, transfer, and removal of a heavy metal (i.e., lead) and its subsequent recovery for recycling purposes. Microbots’ structure consists of nanosized multilayers of graphene oxide, nickel, and platinum, providing different functionalities. The outer layer of graphene oxide captures lead on the surface, and the inner layer of platinum functions as the engine decomposing hydrogen peroxide fuel for self-propulsion, while the middle layer of nickel enables external magnetic control of the microbots. Mobile GOx-microbots remove lead 10 times more efficiently than nonmotile GOx-microbots, cleaning water from 1000 ppb down to below 50 ppb in 60 min. Furthermore, after chemical detachment of lead from the surface of GOx-microbots, the microbots can be reused. Finally, we demonstrate the magnetic control of the GOx-microbots inside a microfluidic system as a proof-of-concept for automatic microbots-based system to remove and recover heavy metals. PB American Chemical Society SN 1530-6984 YR 2016 FD 2016 LK https://hdl.handle.net/20.500.14352/94026 UL https://hdl.handle.net/20.500.14352/94026 LA eng NO Graphene-Based Microbots for Toxic Heavy Metal Removal and Recovery from WaterDiana Vilela, Jemish Parmar, Yongfei Zeng, Yanli Zhao, and Samuel SánchezNano Letters 2016 16 (4), 2860-2866DOI: 10.1021/acs.nanolett.6b00768 NO European Commission NO Alexander von Humboldt Foundation DS Docta Complutense RD 6 abr 2025