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Slowing-down of non-equilibrium concentration fluctuations in confinement

dc.contributor.authorGiraudet, Cédric
dc.contributor.authorBataller, Henri
dc.contributor.authorSun, Yifei
dc.contributor.authorDonev, Aleksander
dc.contributor.authorOrtiz De Zárate Leira, José María
dc.contributor.authorCroccolo, Fabrizio
dc.date.accessioned2023-06-18T06:48:55Z
dc.date.available2023-06-18T06:48:55Z
dc.date.issued2015-09
dc.description© European Physical Society. We acknowledge fruitful discussions with ALBERTO VAILATI, DORIANO BROGIOLI, ROBERTO CERBINO and JAN SENGERS. JMOZ acknowledges support from the UCM-Santander Research Grant PR6/13-18867 during a sabbatical leave in Anglet. AD was supported in part by the U.S. National Science Foundation under grant DMS-1115341 and the Office of Science of the U.S. Department of Energy through Early Career award No. DE-SC0008271.
dc.description.abstractFluctuations in a fluid are strongly affected by the presence of a macroscopic gradient making them long- ranged and enhancing their amplitude. While small-scale fluctuations exhibit diffusive lifetimes, moderate-scale fluctuations live shorter because of gravity. In this letter we explore fluctuations of even larger size, comparable to the extent of the system in the direction of the gradient, and find experimental evidence of a dramatic slowing-down of their dynamics. We recover diffusive behavior for these strongly confined fluctuations, but with a diffusion coefficient that depends on the solutal Rayleigh number. Results from dynamic shadowgraph experiments are complemented by theoretical calculations and numerical simulations based on fluctuating hydrodynamics, and excellent agreement is found. Hence, the study of the dynamics of non-equilibrium fluctuations allows to probe and measure the competition of physical processes such as diffusion, buoyancy and confinement, i.e. the ingredients included in the Rayleigh number, which is the control parameter of our system.
dc.description.departmentDepto. de Estructura de la Materia, Física Térmica y Electrónica
dc.description.facultyFac. de Ciencias Físicas
dc.description.refereedTRUE
dc.description.sponsorshipUnited States Goverment
dc.description.sponsorshipNational Science Foundation (NSF), EE.UU.
dc.description.sponsorshipEarly Career Award, Department of Energy, EE.UU.
dc.description.sponsorshipUniversidad Complutense de Madrid (UCM)
dc.description.sponsorshipBanco Santander Central Hispano (BSCH)
dc.description.statuspub
dc.eprint.idhttps://eprints.ucm.es/id/eprint/34983
dc.identifier.doi10.1209/0295-5075/111/60013
dc.identifier.issn0295-5075
dc.identifier.officialurlhttp://dx.doi.org/10.1209/0295-5075/111/60013
dc.identifier.relatedurlhttp://iopscience.iop.org/
dc.identifier.relatedurlhttp://arxiv.org/pdf/1410.6524
dc.identifier.urihttps://hdl.handle.net/20.500.14352/24282
dc.issue.number6
dc.journal.titleEurophysics letters
dc.language.isoeng
dc.publisherEuropean Physical Society
dc.relation.projectIDPR6/13-18867
dc.relation.projectIDDMS-1115341
dc.relation.projectIDDE-SC0008271
dc.rights.accessRightsopen access
dc.subject.cdu536
dc.subject.keywordLiquid-mixtures
dc.subject.keywordFree diffusion
dc.subject.keywordGravity
dc.subject.keywordFluids
dc.subject.keywordSoret
dc.subject.keywordMicrogravity
dc.subject.keywordShadowgraph
dc.subject.keywordScattering
dc.subject.keywordSchlieren
dc.subject.ucmTermodinámica
dc.subject.unesco2213 Termodinámica
dc.titleSlowing-down of non-equilibrium concentration fluctuations in confinement
dc.typejournal article
dc.volume.number111
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