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Optical absorption in paired correlated random lattices

dc.contributor.authorDomínguez-Adame Acosta, Francisco
dc.contributor.authorMaciá Barber, Enrique Alfonso
dc.contributor.authorSánchez, Angel
dc.date.accessioned2023-06-20T19:12:43Z
dc.date.available2023-06-20T19:12:43Z
dc.date.issued1994-09-01
dc.description© 1994 The American Physical Society. The authors thank Biaachi Mendez for a critical reading of the manuscript. This work is partially supported by UCM under project No. PR161/93-4811. A.S. is supported by a Ministerio de Educacion y Ciencia (Spain)/Fulbright postdoctoral scholarship, by Direccion General de Investigacion Cientifica y Tecnica (Spain) through Project No. PB92-0248, and by the European Community (Union Human Capital and Mobility Programme through Contract No. ERBCHRXCT930413). Work at Los Alamos is performed under the auspices of the U.S. Department of Energy.
dc.description.abstractOptical absorption in a random one-dimensional lattice in the presence of paired correlated disorder is studied. The absorption line shape is evaluated by solving the microscopic equations of motion of the Frenkel-exciton problem in the lattice. We find that paired correlation causes the occurrence of well-defined characteristic lines in the absorption spectra which clearly differ from the case of unpaired correlation. The behavior of the absorption lines as a function of defect concentration is studied in detail. We also show how exciton dynamics can be inferred from experimental data by deriving an analytical expression relating the energy and intensity of lines to the model parameters.
dc.description.departmentDepto. de Física de Materiales
dc.description.facultyFac. de Ciencias Físicas
dc.description.refereedTRUE
dc.description.sponsorshipUCM
dc.description.sponsorshipMinisterio de Educacion y Ciencia (Spain)
dc.description.sponsorshipEuropean Community
dc.description.statuspub
dc.eprint.idhttps://eprints.ucm.es/id/eprint/28072
dc.identifier.doi10.1103/PhysRevB.50.6453
dc.identifier.issn0163-1829
dc.identifier.officialurlhttp://dx.doi.org/10.1103/PhysRevB.50.6453
dc.identifier.relatedurlhttp://journals.aps.org
dc.identifier.urihttps://hdl.handle.net/20.500.14352/59396
dc.issue.number9
dc.journal.titlePhysical Review B
dc.language.isoeng
dc.page.final6456
dc.page.initial6453
dc.publisherAmerican Physical Society
dc.relation.projectIDPR161/93-4811
dc.relation.projectIDPB92-0248
dc.relation.projectIDERBCHRXCT930413
dc.rights.accessRightsopen access
dc.subject.cdu538.9
dc.subject.keywordRandom-Dimer model
dc.subject.keywordFrenkel excitons
dc.subject.keywordSystems
dc.subject.ucmFísica de materiales
dc.titleOptical absorption in paired correlated random lattices
dc.typejournal article
dc.volume.number50
dcterms.references1. D. H. Dunlap, H.-L. Wu, and P. Phillips, Phys. Rev. Lett. 65, 88 (1990). 2. H.-L. Wu and P. Phillips, Phys. Rev. Lett. BB, 1366 (1991). 3. J. C. Flores and M. Hilke, J. Phys. A 28, L1255 (1993). 4. A. Sanchez, E. Macia, and F. Dominguez-Adame, Phys. Rev. B 49, 147 (1994) 5. F. Dominguez-Adame, E. Maciá, and A. Sánchez, Phys. Rev. B 48, 6054 (1993). 6. F. Domínguez-Adame, B. Méndez, A. Sánchez, and E. Maciá, Phys. Rev. B 49, 3839 (1994). 7. D. L. Huber and W. Y. Ching, Chem. Phys. 146, 409 (1990). 8. D. L. Huber and W. Y. Ching, Phys. Rev. B $9, 8652 (1989).
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