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Competing charge ordering and Mott phases in a correlated Sn/Ge(111) two-dimensional triangular lattice

dc.contributor.authorCortés, R
dc.contributor.authorTejeda, A.
dc.contributor.authorLobo Checa, J.
dc.contributor.authorDidiot, C.
dc.contributor.authorKierren, B.
dc.contributor.authorMalterre, D.
dc.contributor.authorMerino, J.
dc.contributor.authorFlores, F.
dc.contributor.authorMichel, E. G.
dc.contributor.authorMascaraque Susunaga, Arantzazu
dc.date.accessioned2023-06-19T13:27:40Z
dc.date.available2023-06-19T13:27:40Z
dc.date.issued2013-09-06
dc.description© 2013 American Physical Society. This work was funded by MICINN (MAT2010-21156-C03-02, MAT2011-22491, and FIS2011-23230), SurMott ANR, and CNRS PICS. We are grateful to L. Patthey of the SIS beamline at the Swiss Light Source for his help during the photoemission experiments.
dc.description.abstractWe take advantage of complementary high-resolution experimental techniques and theoretical tools to get insight into the alpha-Sn/Ge(111) triangular lattice surface consisting of sp electrons. We report a (3 x 3) phase, characterized by a charge ordering settled by electronic correlation, which appears between the known metallic-(3 x 3) and Mott insulator phases. We identify the atomistic mechanism behind the stabilization of this phase and interpret these findings on the basis of theoretical calculations. We disentangle the role of the various degrees of freedom in the stability of the different phases found and describe the stepwise surface changes between the metallic and Mott insulating phases.
dc.description.departmentDepto. de Física de Materiales
dc.description.facultyFac. de Ciencias Físicas
dc.description.refereedTRUE
dc.description.sponsorshipMICINN
dc.description.sponsorshipSurMott ANR
dc.description.sponsorshipCNRS PICS
dc.description.statuspub
dc.eprint.idhttps://eprints.ucm.es/id/eprint/28188
dc.identifier.doi10.1103/PhysRevB.88.125113
dc.identifier.issn1098-0121
dc.identifier.officialurlhttp://dx.doi.org/10.1103/PhysRevB.88.125113
dc.identifier.relatedurlhttp://journals.aps.org
dc.identifier.urihttps://hdl.handle.net/20.500.14352/33766
dc.issue.number12
dc.journal.titlePhysical Review B
dc.language.isoeng
dc.publisherAmerican Physical Society
dc.relation.projectIDMAT2010-21156-C03-02
dc.relation.projectIDMAT2011-22491
dc.relation.projectIDFIS2011-23230
dc.rights.accessRightsopen access
dc.subject.cdu538.9
dc.subject.keywordSurface phase
dc.subject.keywordTransition
dc.subject.keywordTemperature
dc.subject.keywordPb/Ge(111)
dc.subject.keywordSystems
dc.subject.keywordSn/Ge(Iii)
dc.subject.keywordInsulator
dc.subject.keywordDefects
dc.subject.keywordPhonon
dc.subject.keywordState
dc.subject.ucmFísica de materiales
dc.titleCompeting charge ordering and Mott phases in a correlated Sn/Ge(111) two-dimensional triangular lattice
dc.typejournal article
dc.volume.number88
dcterms.references1. N. F. Mott, Metal-Insulator Transitions (Taylor and Francis, London, 1974). 2. F. Gebhard, The Mott Metal-Insulator Transition (Springer, New York, 1997). 3. F. Venturini, M. Opel, T. P. Devereaux, J. K. Freericks, I. Tutto, B. Revaz, E. Walker, H. Berger, L. Forró, and R. Hackl, ´ Phys. Rev. Lett. 89, 107003 (2002). 4. L. Cano-Cortés, J. Merino, and S. Fratini, Phys. Rev. Lett. 105, 036405 (2010). 5. H.-Y. Yang, A. M. Laüchli, F. Mila, and K. P. Schmidt, Phys. Rev. Lett. 105, 267204 (2010). 6. P. A. Lee, N. Nagaosa, and X.-G. Wen, Rev. Mod. Phys. 78, 17 (2006). 7. K. M. F. Kagawa and K. Kanoda, Nature (London) 436, 534 (2005). 8. N. J. DiNardo, T. M. Wong, and E. W. Plummer, Phys. Rev. Lett. 65, 2177 (1990). 9. H. H. Weitering, X. Shi, P. D. Johnson, J. Chen, N. J. DiNardo, and K. Kempa, Phys. Rev. Lett. 78, 1331 (1997). 10. L. A. Cardenas, Y. Fagot-Revurat, L. Moreau, B. Kierren, and D. Malterre, Phys. Rev. Lett. 103, 046804 (2009). 11. L. I. Johansson, F. Owman, and P. Märtensson, Surf. Sci. 360, L478 (1996). 12. R. Cortés, A. Tejeda, J. Lobo, C. Didiot, B. Kierren, D. Malterre, E. G. Michel, and A. Mascaraque, Phys. Rev. Lett. 96, 126103 (2006). 13. J. M. Carpinelli, H. H. Weitering, M. Bartkowiak, R. Stumpf, and E. W. Plummer, Phys. Rev. Lett. 79, 2859 (1997). 14. A. Mascaraque, J. Avila, J. Alvarez, M. C. Asensio, S. Ferrer, and E. G. Michel, Phys. Rev. Lett. 82, 2524 (1999). 15. A. Tejeda, R. Cortés, J. Lobo-Checa, C. Didiot, B. Kierren, D. Malterre, E. G. Michel, and A. Mascaraque, Phys. Rev. Lett. 100, 026103 (2008). 16. S. Modesti, L. Petaccia, G. Ceballos, I. Vobornik, G. Panaccione, G. Rossi, L. Ottaviano, R. Larciprete, S. Lizzit, and A. Goldoni, Phys. Rev. Lett. 98, 126401 (2007). 17. T. Hirahara, T. Komorida, Y. Gu, F. Nakamura, H. Idzuchi, H. Morikawa, and S. Hasegawa, Phys. Rev. B 80, 235419 (2009). 18. G. Profeta and E. Tosatti, Phys. Rev. Lett. 98, 086401 (2007). 19. G. Li, P. Höpner, J. Schäfer, C. Blumenstein, S. Meyer, A. Bostwick, E. Rotenberg, R. Claessen, and W. Hanke, Nat. Commun. 4, 1620 (2013). 20. S. Colonna, F. Ronci, A. Cricenti, and G. LeLay, Phys. Rev. Lett. 101, 186102 (2008). 21. H. Morikawa, S. Jeong, and H. W. Yeom, Phys. Rev. B 78, 245307 (2008). 22. T. Shirasawa, H. Tochihara, K. Kubo, W. Voegeli, and T. Takahashi, Phys. Rev. B 81, 081409(R) (2010). 23. S. Colonna, F. Ronci, A. Cricenti, and G. LeLay, Phys. Rev. Lett. 102, 159602 (2009). 24. H. Morikawa and H. W. Yeom, Phys. Rev. Lett. 102, 159601 (2009). 25. I. Horcas, R. Fernandez, J. M. Gomez-Rodriguez, J. Colchero, J. Gomez-Herrero, and A. M. Baro, Rev. Sci. Instrum. 78, 013705 (2007). 26. A. Ino, C. Kim, M. Nakamura, T. Yoshida, T. Mizokawa, Z.-X. Shen, A. Fujimori, T. Kakeshita, H. Eisaki, and S. Uchida, Phys. Rev. B 62, 4137 (2000). 27. J. Avila, A. Mascaraque, E. G. Michel, M. C. Asensio, G. LeLay, J. Ortega, R. Pérez, and F. Flores, Phys. Rev. Lett. 82, 442 (1999). 28. R. I. G. Uhrberg, H. W. Zhang, and T. Balasubramanian, Phys. Rev. Lett. 85, 1036 (2000). 29. R. I. G. Uhrberg and T. Balasubramanian, Phys. Rev. Lett. 81, 2108 (1998). 30. A. Cano, A. P. Levanyuk, and E. G. Michel, Nanotechnology 16, 325 (2005). 31. A. V. Melechko, J. Braun, H. H. Weitering, and E. W. Plummer, Phys. Rev. B 61, 2235 (2000). 32. A. Cano, A. P. Levanyuk, and E. G. Michel, Z. Kristallogr. 220, 663 (2005). 33. R. M. Feenstra, S. Gaan, G. Meyer, and K. H. Rieder, Phys. Rev. B 71, 125316 (2005). 34. D. M. Riffe and G. K. Wertheim, Phys. Rev. B 61, 2302 (2000). 35. R. Pérez, J. Ortega, and F. Flores, Phys. Rev. Lett. 86, 4891 (2001). 36. D. Farías, W. Kaminski, J. Lobo, J. Ortega, E. Hulpke, R. Pérez, F. Flores, and E. G. Michel, Phys. Rev. Lett. 91, 016103 (2003). 37. E. Pehlke and M. Scheffler, Phys. Rev. Lett. 71, 2338 (1993). 38. J. Ortega, R. Pérez, and F. Flores, J. Phys.: Condens. Matter 12, L21 (2000). 39. S. de Gironcoli, S. Scandolo, G. Ballabio, G. Santoro, and E. Tosatti, Surf. Sci. 454-456, 172 (2000). 40. O. Pulci, M. Marsili, P. Gori, M. Palummo, A. Cricenti, F. Bechstedt, and R. del Sole, Appl. Phys. A 85, 361 (2006). 41. F. Flores, J. Ortega, R. Pérez, A. Charrier, F. Thibaudau, J.- M. Deveber, and J.-M. Themlin, Prog. Surf. Sci. 67, 299 (2001). 42. X. Y. Zhang, M. J. Rozenberg, and G. Kotliar, Phys. Rev. Lett. 70, 1666 (1993). 43. P. Hohenberg and W. Kohn, Phys. Rev. 136, B864 (1964). 44. L. Fritsche, Phys. Rev. B 33, 3976 (1986). 45. Note that the quoted value is slightly larger than the value determined from Fermi surface analysis in Ref. 46, which is attributed to the different method used. 46. A. Tejeda, R. Cortés, J. Lobo, E. G. Michel, and A. Mascaraque, J. Phys.: Condens. Matter 19, 355008 (2007). 47A. Georges, G. Kotliar, W. Krauth, and M. J. Rozenberg, Rev. Mod. Phys. 68, 13 (1996). 48. Upon cooling at 77 K, local COI-(3 × 3) regions are observed (above the transition temperature determined from an averaging technique like photoemission). STS from these areas is shown as it exhibits better defined features than at lower temperatures.
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relation.isAuthorOfPublication9d984e3c-69fb-476e-af0b-5134c4d26028
relation.isAuthorOfPublication.latestForDiscovery9d984e3c-69fb-476e-af0b-5134c4d26028

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