Permanganate loaded Ca-Al-LDH coating for active corrosion protection of 2024-T3 alloy
| dc.contributor.author | Olmo Martínez, Rubén del | |
| dc.contributor.author | Mohedano Sánchez, Marta | |
| dc.contributor.author | Matykina, Endzhe | |
| dc.contributor.author | Arrabal Durán, Raúl | |
| dc.date.accessioned | 2023-06-22T10:40:50Z | |
| dc.date.available | 2023-06-22T10:40:50Z | |
| dc.date.issued | 2022-02-01 | |
| dc.description.abstract | Ca-Al-Layered Double Hydroxide (Ca-Al-LDH) coating was explored on 2024-T3 aluminium alloy by in situ growth methodology following a 1 h treatment at atmospheric pressure. Mn-based species were successfully incorporated into the Ca-Al-LDH structure by a low-temperature post-treatment (Ca-Al-LDH-Mn). Both LDH coatings disclosed a flaky-like morphology and low thickness (~0.6 µm). Ca-Al-LDH-Mn coating showed optimal paint adhesion and the highest long-term corrosion resistance in 3.5 wt% NaCl solution. Evaluation of scribed LDH specimens by SEM/EDS techniques up to 7 days of immersion in 3.5 wt% NaCl solution revealed that the presence of Mn species in the Ca-Al-LDH-Mn provided active corrosion protection. | |
| dc.description.department | Depto. de Ingeniería Química y de Materiales | |
| dc.description.faculty | Fac. de Ciencias Químicas | |
| dc.description.refereed | TRUE | |
| dc.description.sponsorship | Ministerio de Ciencia e Innovación (MICINN)/FEDER | |
| dc.description.sponsorship | Comunidad de Madrid | |
| dc.description.sponsorship | Ministerio de Ciencia e Innovación (MICINN) | |
| dc.description.status | pub | |
| dc.eprint.id | https://eprints.ucm.es/id/eprint/70909 | |
| dc.identifier.doi | 10.1016/j.corsci.2022.110144 | |
| dc.identifier.issn | 0010-938X | |
| dc.identifier.officialurl | https://doi.org/10.1016/j.corsci.2022.110144 | |
| dc.identifier.relatedurl | https://www.sciencedirect.com/science/article/pii/S0010938X22000622 | |
| dc.identifier.uri | https://hdl.handle.net/20.500.14352/71338 | |
| dc.journal.title | Corrosion Science | |
| dc.language.iso | eng | |
| dc.page.initial | 110144 | |
| dc.publisher | Elsevier | |
| dc.relation.projectID | PROFABRICAD (RTI2018-096391-B-C33); | |
| dc.relation.projectID | ADITIMAT-CM (S2018/NMT-4411) | |
| dc.relation.projectID | (RYC-2017-21843) | |
| dc.rights | Atribución-NoComercial-SinDerivadas 3.0 España | |
| dc.rights.accessRights | open access | |
| dc.rights.uri | https://creativecommons.org/licenses/by-nc-nd/3.0/es/ | |
| dc.subject.cdu | 620 | |
| dc.subject.keyword | 2024-T3 | |
| dc.subject.keyword | Aluminium | |
| dc.subject.keyword | Layered double hydroxides | |
| dc.subject.keyword | LDH | |
| dc.subject.keyword | Corrosion inhibitors | |
| dc.subject.keyword | Active corrosion protection | |
| dc.subject.ucm | Materiales | |
| dc.subject.unesco | 3312 Tecnología de Materiales | |
| dc.title | Permanganate loaded Ca-Al-LDH coating for active corrosion protection of 2024-T3 alloy | |
| dc.type | journal article | |
| dc.volume.number | 198 | |
| dcterms.references | C. Vargel Chapter F.1 - Protection of aluminium C. Vargel (Ed.), Corrosion of Aluminium (second ed.), Elsevier, Amsterdam (2020), pp. 383-443 ArticleDownload PDFView Record in ScopusGoogle Scholar [2] S. Cramer ASM handbook, volume 13A - corrosion: fundamentals Testing, and Protection, ASM International, (2010) 07-06 Google Scholar [3] S. Kulinich, A. Akhtar On conversion coating treatments to replace chromating for Al Alloys: recent developments and possible future directions Russ. J. Non Ferr. Met., 53 (2012), pp. 176-203 View Record in ScopusGoogle Scholar [4] LANXESS Surf. Treat. Appl. Aeronaut. Aerosp. Ind. (137) (2018) [5] T.P. Schuman Chapter 17 - Protective coatings for aluminum alloys M. Kutz (Ed.), Handbook of Environmental Degradation of Materials, William Andrew Publishing, Norwich, NY (2005), pp. 345-366 ArticleDownload PDFView Record in ScopusGoogle Scholar [6] D.C. Beelen, P. Rouw, R. Boomgaard, K. Zabel Aviox CF Primer: a new generation primer for aircraft maintenance Pigment Resin Technol., 27 (1998), pp. 28-33 Google Scholar [7] A.E. Hughes, T.G. Harvey, N. Birbilis, A. Kumar, R.G. Buchheit 7 - Coatings for corrosion prevention based on rare earths M. Forsyth, B. Hinton (Eds.), Rare Earth-Based Corrosion Inhibitors, Woodhead Publishing (2014), pp. 186-232 ArticleDownload PDFCrossRefView Record in ScopusGoogle Scholar [8] D. Mitton, A. Carangelo, A. Acquesta, T. Monetta, M. Curioni, F. Bellucci Selected Cr(VI) replacement options for aluminum alloys: a literature survey Corros. Rev., 35 (2017) Google Scholar [9] J. Qi, T. Hashimoto, J.R. Walton, X. Zhou, P. Skeldon, G. Thompson Trivalent chromium conversion coating formation on aluminium Surf. Coat. Technol., 280 (2015), pp. 317-329 ArticleDownload PDFView Record in ScopusGoogle Scholar [10] M.G.S. Ferreira, M.L. Zheludkevich, J. Tedim Advanced protective coatings for aeronautical applications Nanocoatings Ultra Thin Films: Technol. Appl. (2011), pp. 235-279 ArticleDownload PDFCrossRefView Record in ScopusGoogle Scholar [11] X. Guo, F. Zhang, D. Evans, X. Duan, Layered double hydroxide films: Synthesis, properties and applications, Chemical communications (Cambridge, England), 46 (2010) 5197–5210. Google Scholar [12] K.A. Yasakau, M.L. Zheludkevich, M.G.S. Ferreira Corrosion and corrosion protection of aluminum alloys K. Wandelt (Ed.), Encyclopedia of Interfacial Chemistry, Elsevier, Oxford (2018), pp. 115-127 ArticleDownload PDFView Record in ScopusGoogle Scholar [13] D.G. Evans, R.C.T. Slade Structural aspects of layered double hydroxides X. Duan, D.G. Evans (Eds.), Layered Double Hydroxides, Springer Berlin Heidelberg, Berlin, Heidelberg (2006), pp. 1-87 Google Scholar [14] J. Tedim, M.L. Zheludkevich, A.C. Bastos, A.N. Salak, A.D. Lisenkov, M.G.S. Ferreira Influence of preparation conditions of Layered Double Hydroxide conversion films on corrosion protection Electrochim. Acta, 117 (2014), pp. 164-171 ArticleDownload PDFView Record in ScopusGoogle Scholar [15] J. Tedim, A.I. Kuznetsova, A. Salak, M. Montemor, D. Snihirova, M. Pilz, M.L. Zheludkevich, M. Ferreira Zn-Al layered double hydroxides as chloride nanotraps in active protective coatings Corros. Sci., 55 (2012), pp. 1-4 ArticleDownload PDFView Record in ScopusGoogle Scholar [16] M.L. Zheludkevich, S.K. Poznyak, L.M. Rodrigues, D. Raps, T. Hack, L.F. Dick, T. Nunes, M.G.S. Ferreira Active protection coatings with layered double hydroxide nanocontainers of corrosion inhibitor Corros. Sci., 52 (2010), pp. 602-611 ArticleDownload PDFView Record in ScopusGoogle Scholar [17] A.C. Bouali, M. Serdechnova, C. Blawert, J. Tedim, M.G.S. Ferreira, M.L. Zheludkevich Layered double hydroxides (LDHs) as functional materials for the corrosion protection of aluminum alloys: a review Appl. Mater. Today, 21 (2020), Article 100857 ArticleDownload PDFView Record in ScopusGoogle Scholar [18] J. Tedim, M.L. Zheludkevich, A. Salak, A.D. Lisenkov, M. Ferreira Nanostructured LDH-container layer with active protection functionality J. Mater. Chem., 21 (2011), pp. 15464-15470 View PDFCrossRefView Record in ScopusGoogle Scholar [19] J. Wu, D. Peng, Y. He, X. Du, Z. Zhang, B. Zhang, X. Li, Y. Huang In situ formation of decavanadate-intercalated layered double hydroxide films on AA2024 and their anti-corrosive properties when combined with hybrid sol gel films Materials (2017), p. 426 View PDFCrossRefView Record in ScopusGoogle Scholar [20] J. Tedim, M.L. Zheludkevich, A.C. Bastos, A.N. Salak, J. Carneiro, F. Maia, A.D. Lisenkov, A.B. Oliveira, M.G.S. Ferreira Effect of surface treatment on the performance of LDH conversion films ECS Electrochem. Lett., 3 (2014), pp. C4-C8 View Record in ScopusGoogle Scholar [21] Y. Zhang, J. Liu, l Yingdong, M. Yu, S. Li, B. Xue Fabrication of inhibitor anion-intercalated layered double hydroxide host films on aluminum alloy 2024 and their anticorrosion properties J. Coat. Technol. Res., 12 (2015), pp. 293-302 View PDFCrossRefGoogle Scholar [22] Y. Zhang, Y. Li, Y. Ren, H. Wang, F. Chen Double-doped LDH films on aluminum alloys for active protection Mater. Lett., 192 (2017), pp. 33-35 ArticleDownload PDFCrossRefGoogle Scholar [23] Y. Zhang, P. Yu, J. Wang, Y. Li, F. Chen, K. Wei, Y. Zuo LDHs/graphene film on aluminum alloys for active protection Appl. Surf. Sci., 433 (2018), pp. 927-933 ArticleDownload PDFGoogle Scholar [24] S.U. Ofoegbu, F.A.O. Fernandes, A.B. Pereira The sealing step in aluminum anodizing: a focus on sustainable strategies for enhancing both energy efficiency and corrosion resistance Coatings, 10 (2020), p. 226 View PDFCrossRefView Record in ScopusGoogle Scholar [25] F. Millange, R. Walton, L. Lei, D. O’Hare Efficient separation of terephthalate and phthalate anions by selective ion-exchange intercalation in the layered double hydroxide Ca 2 Al(OH) 6·NO 3·2H 2 O Chem. Mater., 12 (2000), pp. 1990-1994 View PDFView Record in ScopusGoogle Scholar [26] M. Meyn, K. Beneke, G. Lagaly Anion-exchange reactions of layered double hydroxides Inorg. Chem., 29 (1990), pp. 5201-5207 View PDFCrossRefView Record in ScopusGoogle Scholar [27] A.V. Radha, P. Vishnu Kamath, C. Shivakumara Mechanism of the anion exchange reactions of the layered double hydroxides (LDHs) of Ca and Mg with Al Solid State Sci., 7 (2005), pp. 1180-1187 ArticleDownload PDFView Record in ScopusGoogle Scholar [28] M. Iqbal, L. Sun, A. LaChance, H. Ding, M. Fedel In situ growth of CaAl-NO3--layered double hydroxide directly on aluminum alloy for corrosion resistance Dalton Trans., 49 (2019) Google Scholar [29] A. Pardo, S. Feliu, M. Merino, R. Arrabal, E. Matykina XPS study of chemical changes on the La/Ce treated surface of A361 aluminium alloy exposed to air at temperatures up to 500∘C Adv. Mater. Sci. Eng. (2009) Google Scholar [30] G. Yoganandan, J.N. Balaraju, V.K. William Grips The surface and electrochemical analysis of permanganate based conversion coating on alclad and unclad 2024 alloy Appl. Surf. Sci., 258 (2012), pp. 8880-8888 ArticleDownload PDFView Record in ScopusGoogle Scholar [31] S.A. Kulinich, M. Farzaneh, X.W. Du Growth of corrosion-resistant manganese oxide coatings on an aluminum alloy Inorg. Mater., 43 (2007), pp. 956-963 View Record in ScopusGoogle Scholar [32] S.B. Madden, J.R. Scully Inhibition of AA2024-T351 corrosion using permanganate J. Electrochem. Soc., 161 (2014), pp. C162-C175 View PDFCrossRefView Record in ScopusGoogle Scholar [33] B. Dou, Y. Wang, T. Zhang, B. Liu, Y. Shao, G. Meng, F. Wang Growth behaviors of layered double hydroxide on microarc oxidation film and anti-corrosion performances of the composite film J. Electrochem. Soc., 163 (2016), pp. C917-C927 View PDFCrossRefView Record in ScopusGoogle Scholar [34] F. Zhang, C.L. Zhang, L. Song, R.C. Zeng, Z.G. Liu, H.Z. Cui Corrosion of in-situ grown MgAl-LDH coating on aluminum alloy Trans. Nonferrous Met. Soc. China, 25 (2015), pp. 3498-3504 ArticleDownload PDFView Record in ScopusGoogle Scholar [35] K.M. Dietmann, T. Linke, M.D. Nogal Sánchez, J.L. Pérez Pavón, V. Rives Layered double hydroxides with intercalated permanganate and peroxydisulphate anions for oxidative removal of chlorinated organic solvents contaminated water Minerals, 10 (2020) Google Scholar [36] J.D. Hem Chemical equilibria and rates of manganese oxidation Geological Survey Water-Supply Paper, 1667, united states government printing office,, washington (1963) Google Scholar [37] M. Szabados, R. Mészáros, S. Erdei, Z. Kónya, Á. Kukovecz, P. Sipos, I. Pálinkó Ultrasonically-enhanced mechanochemical synthesis of CaAl-layered double hydroxides intercalated by a variety of inorganic anions Ultrason. Sonochem., 31 (2016), pp. 409-416 ArticleDownload PDFView Record in ScopusGoogle Scholar [38] E. Heraldy, K.D. Nugrahaningtyas, Heriyanto, X-ray Diffraction Analysis on Post Treatment of Ca-Mg-Al-Layered Double Hydroxide Slurry, IOP Conference Series: Materials Science and Engineering, 176 (2017) 012020. Google Scholar [39] G. Varga, Á. Kukovecz, Z. Kónya, L. Korecz, S. Muráth, Z. Csendes, G. Peintler, S. Carlson, P. Sipos, I. Pálinkó Mn(II)-amino acid complexes intercalated in CaAl-layered double hydroxide - well-characterized, highly efficient, recyclable oxidation catalysts J. Catal., 335 (2016), pp. 125-134 ArticleDownload PDFView Record in ScopusGoogle Scholar [40] C. Yang, L. Liao, G. Lv, L. Wu, L. Mei, Z. Li Synthesis and characterization of Mn intercalated Mg-Al hydrotalcite J. Colloid Interface Sci., 479 (2016), pp. 115-120 ArticleDownload PDFView Record in ScopusGoogle Scholar [41] J.L. Milagres, C.R. Bellato, R.S. Vieira, S.O. Ferreira, C. Reis Preparation and evaluation of the Ca-Al layered double hydroxide for removal of copper(II), nickel(II), zinc(II), chromium(VI) and phosphate from aqueous solutions J. Environ. Chem. Eng., 5 (2017), pp. 5469-5480 ArticleDownload PDFView Record in ScopusGoogle Scholar [42] A. Korchef, M. Touaibi Effect of pH and temperature on calcium carbonate precipitation by CO2 removal from iron-rich water Water Environ., 34 (2020), pp. 331-341 View PDFCrossRefView Record in ScopusGoogle Scholar [43] M.A. Iqbal, M. Secchi, M.A. Iqbal, M. Montagna, C. Zanella, M. Fedel MgAl-LDH/graphene protective film: Insight into LDH-graphene interaction Surf. Coat. Technol., 401 (2020), Article 126253 ArticleDownload PDFView Record in ScopusGoogle Scholar [44] A.C. Bouali, M.H. Iuzviuk, M. Serdechnova, K.A. Yasakau, D. Drozdenko, A. Lutz, K. Fekete, G. Dovzhenko, D.C.F. Wieland, H. Terryn, M.G.S. Ferreira, I.A. Zobkalo, M.L. Zheludkevich Mechanism of LDH direct growth on aluminum alloy surface: a kinetic and morphological approach J. Phys. Chem. C., 125 (2021), pp. 11687-11701 View PDFCrossRefView Record in ScopusGoogle Scholar [45] M. Shabanian, M. Hajibeygi, A. Raeisi 2 - FTIR characterization of layered double hydroxides and modified layered double hydroxides S. Thomas, S. Daniel (Eds.), Layered Double Hydroxide Polymer Nanocomposites, Woodhead Publishing, New York (2020), pp. 77-101 ArticleDownload PDFView Record in ScopusGoogle Scholar [46] S. Aisawa, H. Hirahara, H. Uchiyama, S. Takahashi, E. Narita Synthesis and thermal decomposition of Mn–Al layered double hydroxides J. Solid State Chem., 167 (2002), pp. 152-159 ArticleDownload PDFView Record in ScopusGoogle Scholar [47] J.T. Kloprogge, R.L. Frost Fourier transform infrared and Raman spectroscopic study of the local structure of Mg-, Ni-, and Co-Hydrotalcites J. Solid State Chem., 146 (1999), pp. 506-515 ArticleDownload PDFView Record in ScopusGoogle Scholar [48] H. Chen, J. He Facile synthesis of monodisperse manganese oxide nanostructures and their application in water treatment J. Phys. Chem. C., 112 (2008), pp. 17540-17545 View PDFCrossRefView Record in ScopusGoogle Scholar [49] M. Zheng, H. Zhang, X. Gong, R. Xu, Y. Xiao, H. Dong, X. Liu, Y. Liu A simple additive-free approach for the synthesis of uniform manganese monoxide nanorods with large specific surface area Nanoscale Res. Lett., 8 (2013), p. 166 View PDFCrossRefView Record in ScopusGoogle Scholar [50] Y. Wang, Y. Zhang, B. Zhou, C. Li, F. Gao, X. Wang, D. Liang, Y. Wei In-situ observation of the growth behavior of ZnAl layered double hydroxide film using EQCM Mater. Des., 180 (2019), Article 107952 ArticleDownload PDFView Record in ScopusGoogle Scholar [51] J. Zhu, Z. Zhu, H. Zhang, H. Lu, Y. Qiu Efficient degradation of organic pollutants by peroxymonosulfate activated with MgCuFe-layered double hydroxide RSC Adv., 9 (2019), pp. 2284-2291 View PDFCrossRefView Record in ScopusGoogle Scholar [52] Y. Zou, X. Wang, F. Wu, S. Yu, Y. Hu, W. Song, Y. Liu, H. Wang, T. Hayat, X. Wang Controllable synthesis of Ca-Mg-Al layered double hydroxides and calcined layered double oxides for the efficient removal of U(VI) from wastewater solutions ACS Sustain. Chem. Eng., 5 (2017), pp. 1173-1185 View PDFCrossRefView Record in ScopusGoogle Scholar [53] L. He-Ming, Y.-X. Sun, F. Zhang, D.-Y. Zhang, Y.-F. Zhang Preparation and electrochemical applications of spherical maltose-based templated carbon/MnOx composite materials Electrochim. Acta, 148 (2014) Google Scholar [54] Z. Khan, S. Ahmed Al- Thabaiti, A. Yousif Obaid, Z.A. Khan MnO2 nanostructures of different morphologies from amino acids–MnO4− reactions in aqueous solutions Colloids Surf. B: Biointerfaces, 81 (2010), pp. 381-384 ArticleDownload PDFView Record in ScopusGoogle Scholar [55] M.A. Iqbal, L. Sun, A.T. Barrett, M. Fedel Layer. Double Hydroxide Prot. Films Dev. Alum. Alum. Alloy.: Synth. Methods Anti-Corros. Mech., 10 (2020), p. 428 View PDFCrossRef [56] J. Wu, D. Peng, Y. He, X. Du, Z. Zhang, B. Zhang, X. Li, Y. Huang In situ formation of decavanadate-intercalated layered double hydroxide films on AA2024 and their anti-corrosive properties when combined with hybrid sol gel films Materials, 10 (2017) Google Scholar [57] J. Tedim, A.C. Bastos, S. Kallip, M.L. Zheludkevich, M.G.S. Ferreira Corrosion protection of AA2024-T3 by LDH conversion films. Analysis of SVET results Electrochim. Acta, 210 (2016), pp. 215-224 ArticleDownload PDFView Record in ScopusGoogle Scholar [58] H.A. Swain, C. Lee, R.B. Rozelle Determination of the solubility of manganese hydroxide and manganese dioxide at 25.deg. by atomic absorption spectrometry Anal. Chem., 47 (1975), pp. 1135-1137 View PDFCrossRefView Record in ScopusGoogle Scholar [59] S.-Y. Jian, C.-Y. Yang, J.-K. Chang Robust corrosion resistance and self-healing characteristics of a novel Ce / Mn conversion coatings on EV31 magnesium alloys Appl. Surf. Sci., 510 (2020), Article 145385 ArticleDownload PDFView Record in ScopusGoogle Scholar [60] N. Takeno Atlas of Eh-pH diagrams - intercomparison of thermodynamic databases GSJ, Geological Survey of Japan (2005) (AIS) Google Scholar | |
| dspace.entity.type | Publication | |
| relation.isAuthorOfPublication | 160ef5bd-2d04-4f6c-b028-cb7ce4cf8d38 | |
| relation.isAuthorOfPublication | 427b12dd-40e9-49e6-a8fe-d41e79a056ff | |
| relation.isAuthorOfPublication | 6a953ac5-3b84-40fc-a995-2a00ac938151 | |
| relation.isAuthorOfPublication.latestForDiscovery | 160ef5bd-2d04-4f6c-b028-cb7ce4cf8d38 |
Download
Original bundle
1 - 1 of 1
