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Separation and fractionation of order and disorder in highly polydisperse systems

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dc.contributor.authorFernández Pérez, Luis Antonio
dc.contributor.authorMartín Mayor, Víctor
dc.contributor.authorSeoane Bartolomé, Beatriz
dc.contributor.authorVerrocchio, P.
dc.date.accessioned2023-06-20T04:13:09Z
dc.date.available2023-06-20T04:13:09Z
dc.date.issued2010-08-05
dc.description© 2010 The American Physical Society.We acknowledge BIFI cluster and CINECA for 2 x 10^(5) h of computer time. We have been partly supported through Research Contracts No. FIS2006-08533, No. FIS2009-12648-C03-01, and No. FIS2008-01323 MICINN, Spain and by UCM-Banco de Santander Grant No. GR58/ 08. B.S. was supported by the FPU program (Spain).
dc.description.abstractWe study a polydisperse soft-spheres model for colloids by means of microcanonical Monte Carlo simulations. We consider a polydispersity as high as 24%. Although solidification occurs, neither a crystal nor an amorphous state are thermodynamically stable. A finite size scaling analysis reveals that in the thermodynamic limit: a the fluid-solid transition is rather a crystal-amorphous phase-separation, b such phase-separation is preceded by the dynamic glass transition, and c small and big particles arrange themselves in the two phases according to a complex pattern not predicted by any fractionation scenario.
dc.description.departmentDepto. de Física Teórica
dc.description.facultyFac. de Ciencias Físicas
dc.description.refereedTRUE
dc.description.sponsorshipMinisterio de Ciencia e Innovación (MICINN)
dc.description.sponsorshipUCM-Banco de Santander
dc.description.sponsorshipFPU program (Spain)
dc.description.statuspub
dc.eprint.idhttps://eprints.ucm.es/id/eprint/37828
dc.identifier.doi10.1103/PhysRevE.82.021501
dc.identifier.issn1539-3755
dc.identifier.officialurlhttp://doi.org/10.1103/PhysRevE.82.021501
dc.identifier.relatedurlhttp://journals.aps.org/
dc.identifier.urihttps://hdl.handle.net/20.500.14352/45055
dc.issue.number2
dc.journal.titlePhysical review E
dc.language.isoeng
dc.publisherAmerican Physical Society
dc.relation.projectIDFIS2006-08533
dc.relation.projectIDFIS2009-12648-C03-01
dc.relation.projectIDFIS2008-01323
dc.relation.projectIDGR58/08
dc.rights.accessRightsopen access
dc.subject.cdu51-73
dc.subject.cdu53
dc.subject.keywordMonte-Carlo method
dc.subject.keywordCrystal nucleation
dc.subject.keywordHard-spheres
dc.subject.keywordGlasses
dc.subject.keywordLiguids.
dc.subject.ucmFísica (Física)
dc.subject.ucmFísica-Modelos matemáticos
dc.subject.unesco22 Física
dc.titleSeparation and fractionation of order and disorder in highly polydisperse systems
dc.typejournal article
dc.volume.number82
dcterms.references1) P. N. Pusey, W. van Megen, Nature (London), 320, 340, 1986. 2) P. Bartlett, J. Chem. Phys., 109, 10970, 1998. 3) D. A. Kofke, P. G. Bolhuis, Phys. Rev. E, 59, 618, 1999. 4) S. Auer, D. Frenkel, Nature (London), 413, 711, 2001. 5) M. Fasolo, P. Sollich, Phys. Rev. E, 70, 041410, 2004. 6) R. P. A. Dullens, W. K. Kegel, Phys. Rev. Lett., 92, 195702, 2004. 7) P. Chaudhuri, S. Karmakar, C. Dasgupta, H. R. Krishnamurthy, A. K. Sood, Phys. Rev. Lett., 95, 248301, 2005. 8) L. A. Fernández, V. Martín-Mayor, P. Verrocchio, Phys. Rev. Lett., 98, 085702, 2007. 9) G. Brambilla, D. El Masri, M. Pierno, L. Berthier, L. Cipelletti, G. Petekidis, A. B. Schofield, Phys. Rev. Lett., 102, 085703, 2009. 10) E. Zaccarelli, C. Valeriani, E. Sanz, W. C. K. Poon, M. E. Cates, P. N. Pusey, Phys. Rev. Lett., 103, 135704, 2009. 11) L. A. Fernández, V. Martín-Mayor, P. Verrocchio, The Xth International Workshop on Disordered Systems (Taylor & Francis, New York), 2007, Vol. 87, pp. 581–586. 12) Q. Yan, J. J. de Pablo, Phys. Rev. Lett., 90, 035701, 2003. 13) J. P. Hansen, I. R. McDonald, Theory of Simple Liquids (Academic Press, San Diego), 1986. 14) L. Santen, W. Krauth, e-print arXiv:cond-mat/0107459. 15) L. Berthier, W. Kob, J. Phys.: Condens. Matter, 19, 205130, 2007. 16) N. B. Simeonova, W. K. Kegel, Phys. Rev. Lett., 93, 035701, 2004. 17) W. Gotze, L. Sjogren, Rep. Prog. Phys., 55, 241 1992. 18) V. N. Novikov, A. P. Sokolov, Phys. Rev. E, 67, 031507, 2003. 19) R. Lustig, J. Chem. Phys., 109, 8816, 1998. 20) V. Martín-Mayor, Phys. Rev. Lett., 98, 137207, 2007. 21) P. J. Steinhardt, D. R. Nelson, M. Ronchetti, Phys. Rev. B, 28, 784, 1983. 22) P. Rein ten Wolde, M. J. Ruiz-Montero, D. Frenkel, J. Chem. Phys., 104, 9932, 1996. 23) L. A. Fernández, A. Gordillo-Guerrero, V. Martín Mayor, J. J. Ruiz-Lorenzo, Phys. Rev. Lett., 100, 057201, 2008. 24) K. Hukushima, K. Nemoto, J. Phys. Soc. Jpn., 65, 1604, 1996. 25) E. Marinari, in Advances in Computer Simulation, edited by J. Kerstész and I. Kondor (Springer-Verlag, Berlin), 1998. 26) T. S. Grigera, G. Parisi, Phys. Rev. E, 63, 045102, 2001. 27) Q. Yan, T. S. Jain, J. J. de Pablo, Phys. Rev. Lett., 92, 235701, 2004. 28) L. A. Fernández, V. Martín-Mayor, S. Pérez-Gaviro, A. Tarancón, A. P. Young, Phys. Rev. B, 80, 024422, 2009. 29) D. P. Landau, K. Binder, A Guide to Monte Carlo Simulations in Statistical Physics (Cambridge University Press, Cambridge, England), 2000. 30) P. Sollich, N. B. Wilding, Phys. Rev. Lett., 104, 118302, 2010. 31) B. Bernu, J. P. Hansen, Y. Hiwatari, G. Pastore, Phys. Rev. A, 36, 4891, 1987. 32) C. C. Yu, H. M. Carruzzo, Phys. Rev. E, 69, 051201, 2004. 33) L. A. Fernández, V. Martín-Mayor, P. Verrocchio, Phys. Rev. E, 73, 020501, 2006.
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