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Quest for order in chaos: hidden repulsive level statistics in disordered quantum nanoaggregates

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dc.contributor.authorAugulis, R.
dc.contributor.authorMalyshev, Andrey
dc.contributor.authorPugžlys, A.
dc.contributor.authorLoosdrecht, P. H. M. van
dc.contributor.authorKnoester, J.
dc.date.accessioned2023-06-20T00:36:02Z
dc.date.available2023-06-20T00:36:02Z
dc.date.issued2010-10-07
dc.description© ACS. This work is part of the research program of the Stichting voor Fundamenteel Onderzoek der Materie (FOM), which is financially supported by the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO). A. V. M. and V. A. M. acknowledge support from NanoNed, a national nanotechnology programme coordinated by the Dutch Ministry of Economic Affairs. A. V. M. also acknowledges support from the program Ramón y Cajal (Ministerio de Ciencia y Tecnología de España).
dc.description.abstractThe local distribution of exciton levels in disordered cyanine-dye-based molecular nanoaggregates has been elucidated using fluorescence line narrowing spectroscopy. The observation of a Wigner-Dyson-type level spacing distribution provides direct evidence of the existence of level repulsion of strongly overlapping states in the molecular wires, which is important for the understanding of the level statistics, and therefore the functional properties, of a large variety of nanoconfined systems.
dc.description.departmentDepto. de Física de Materiales
dc.description.facultyFac. de Ciencias Físicas
dc.description.refereedTRUE
dc.description.sponsorshipMinisterio de Ciencia e Innovación (MICINN)
dc.description.sponsorshipNederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO)
dc.description.sponsorshipNanoNed-Dutch Ministry of Economic Affairs
dc.description.statuspub
dc.eprint.idhttps://eprints.ucm.es/id/eprint/45715
dc.identifier.doi10.1021/jz101003j
dc.identifier.issn1948-7185
dc.identifier.officialurlhttp://dx.doi.org/10.1021/jz101003j
dc.identifier.relatedurlhttp://pubs.acs.org
dc.identifier.urihttps://hdl.handle.net/20.500.14352/42783
dc.issue.number19
dc.journal.titleJournal of physical chemistry letters
dc.language.isoeng
dc.page.final2916
dc.page.initial2911
dc.publisherACS
dc.rights.accessRightsopen access
dc.subject.cdu538.9
dc.subject.keywordLocalized frenkel excitons
dc.subject.keywordLow-temperature
dc.subject.keywordRayleigh-scattering
dc.subject.keywordOptical-properties
dc.subject.keywordNanoscale systems
dc.subject.keywordEnergy
dc.subject.keywordSpectroscopy
dc.subject.keywordRelaxation
dc.subject.keywordProteins
dc.subject.keywordInsights
dc.subject.ucmFísica de materiales
dc.subject.ucmFísica del estado sólido
dc.subject.unesco2211 Física del Estado Sólido
dc.titleQuest for order in chaos: hidden repulsive level statistics in disordered quantum nanoaggregates
dc.typejournal article
dc.volume.number1
dspace.entity.typePublication
relation.isAuthorOfPublicationb2abe0ef-0417-4f43-8dce-55d3205e22ec
relation.isAuthorOfPublication.latestForDiscoveryb2abe0ef-0417-4f43-8dce-55d3205e22ec

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